Effect of Vapor-Liquid Equilibrium on CO2 Gas Absorption by Amine Peprasine- Ionic liquid Solution Using Central Composite Test Design Method

Document Type : Review Paper

Authors
Soheila Zare 1
Abdolrasoul Pouranfard 2
1 PhD Student, Department of Chemical Engineering, Engineering Faculty, Yasuj University, Yasouj, Iran
2 Assistant Professor, Department of Chemical Engineering, Engineering Faculty, Yasouj University, Yasouj, Iran
20.1001.1/ijge.2023.707975
Abstract
In this research, the absorption of CO2 by an aqueous solution of Amine Piperazine-Ionic liquid was investigated. The Response Surface Method (RSM) based on Central Composite Design (CCD) was used to design experiments, build models, and find optimal operating conditions to achieve optimal responses in the range of used temperature, pressure, and time. The design and optimization of this group of separation units requires to accurate equilibrium and thermodynamic data of vapor-liquid equilibrium. In this study, the optimal loading conditions of CO2 gas were determined using the central composite design (CMD) method. Analysis of the equations performed using quadratic polynomial regression and ANOVA analysis of variance. Enhancement of the pressure and time and reducing the temperature cause increase the solubility of carbon dioxide gas in the amine mixture. The optimal absorption conditions were obtained at pressure 1.6 bar, temperature 21 ℃ and time 1.5 hours. Finally, the mechanism of temperature effect on solubility via Lochatelier’s principle, the effect of pressure on solubility by Henry’s law, and the effect of time on solubility by examining the kinetics of the adsorption reaction was investigated.
Keywords
CO2 gas absorption
Amine Peprasine-Ionic liquid mixture
Vapor-liquid equilibrium
CMD
Subjects
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Iranian Journal of Gas Engineering
Volume 10, Issue 1 - Serial Number 19
September 2023
Pages 80-93

  • Receive Date 12 June 2023
  • Revise Date 27 July 2023
  • Accept Date 19 August 2023